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The charge redistribution upon photoexcitation is investigated for a series of pyrene photoacids to better understand the driving force behind excited-state proton-transfer processes. The changes in e...
Many mixed-valence systems involve two or more states with different electric dipole moments whose magnitudes depend upon the charge transfer distance and the degree of delocalization; these systems c...
Stark spectra have been obtained in the region of absorption by the accessory bacteriochlorophylls (the B-band region around 800 nm) in Rhodobacter sphaeroides reaction centers. The Stark spectra in t...
Resonance Stark effects are nonclassical Stark effects associated with excited-state charge-transfer processes. The theory of resonance Stark effects developed in Part 2 of this series is generalized ...
The vibrational Stark effect measures the effect of an external electric field on the vibrational (IR) spectrum of a molecule. This technique gives quantitative information on the sensitivity of a vib...
We report the first measurement of the vibrational Stark effect in a protein, providing quantitative information on the sensitivity of a vibrational transition to an applied electric field. This can b...
The electronic absorption line shape and Stark spectrum of the lowest energy Q(y)() transition of the special pair in bacterial reaction centers contain a wealth of information on mixing with charge t...
A theory of the resonance Stark effect data reported in part 1 (preceding paper in this issue) is developed. The model used involves a weak charge resonance interaction between the excited state of an...
Higher order Stark spectroscopy has recently been introduced and applied to characterize the electrooptic properties of chromophores in bacterial photosynthetic reaction centers.1 In the course of the...
We present low-temperature Stark measurements on the core light-harvesting complex 1 (LH1) of purple bacteria and the B820 subunit derived from LH1, which is a protein bound Bchl a dimer. It was found...
Stark spectroscopy has been applied to a wide range of molecular systems and materials. A generally useful method for obtaining electronic and vibrational Stark spectra that does not require sophistic...
The electronic structure of donor/acceptor polyenes (merocyanines) is studied by means of electroabsorption (Stark) spectroscopy. Molecules belonging to this class exhibit an extreme variability of th...
Stark Spectroscopy of Donor-Acceptor Polyenes:Correlation with Nonlinear Optical Measurements.
The effects of applied electric fields on the absorption or emission spectrum of a molecule is known as Stark Spectroscopy. This method probes the movement of charge associated with optical excitation...
Stark spectra for nonoriented molecules with typical broad inhomogeneous line widths are obtained by applying an ac electric field and detecting the change in absorbance at the second harmonic of the ...

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